Enhanced CO2 capture capacities and efficiencies with N-doped nanoporous carbons synthesized from solvent-modulated, pyridinedicarboxylate-containing Zn-MOFs

Jongsik Kim; Allen G. Oliver; Jason C. Hicks

doi:10.1039/c5ce00828j

Enhanced CO₂ capture capacities and efficiencies with N-doped nanoporous carbons synthesized from solvent-modulated, pyridinedicarboxylate-containing Zn-MOFs

Jongsik Kim, Allen G. Oliver, Jason C. Hicks

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13 Citations (Scopus)

Abstract

This paper describes the pyrolysis of pyridinedicarboxylate-containing Zn-based metal-organic frameworks (MOFs) to form nanoporous carbons with accessible N dopants to adsorb CO₂. The optimal materials were synthesized using N-heterocycle additives to control the amount of coordinated DMF in the base MOF structure, thereby increasing its thermal stability prior to pyrolysis.

Original language	English
Pages (from-to)	8015-8020
Number of pages	6
Journal	CrystEngComm
Volume	17
Issue number	42
DOIs	https://doi.org/10.1039/c5ce00828j
Publication status	Published - 2015

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© The Royal Society of Chemistry.

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abstract = "This paper describes the pyrolysis of pyridinedicarboxylate-containing Zn-based metal-organic frameworks (MOFs) to form nanoporous carbons with accessible N dopants to adsorb CO2. The optimal materials were synthesized using N-heterocycle additives to control the amount of coordinated DMF in the base MOF structure, thereby increasing its thermal stability prior to pyrolysis.",

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AB - This paper describes the pyrolysis of pyridinedicarboxylate-containing Zn-based metal-organic frameworks (MOFs) to form nanoporous carbons with accessible N dopants to adsorb CO2. The optimal materials were synthesized using N-heterocycle additives to control the amount of coordinated DMF in the base MOF structure, thereby increasing its thermal stability prior to pyrolysis.

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Enhanced CO₂ capture capacities and efficiencies with N-doped nanoporous carbons synthesized from solvent-modulated, pyridinedicarboxylate-containing Zn-MOFs

Abstract

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