Enhanced CO2 capture capacities and efficiencies with N-doped nanoporous carbons synthesized from solvent-modulated, pyridinedicarboxylate-containing Zn-MOFs

Jongsik Kim; Allen G. Oliver; Jason C. Hicks

doi:10.1039/c5ce00828j

Enhanced CO₂ capture capacities and efficiencies with N-doped nanoporous carbons synthesized from solvent-modulated, pyridinedicarboxylate-containing Zn-MOFs

Jongsik Kim
, Allen G. Oliver
, Jason C. Hicks

Research output: Contribution to journal › Article › peer-review

14 Citations (Scopus)

Abstract

This paper describes the pyrolysis of pyridinedicarboxylate-containing Zn-based metal-organic frameworks (MOFs) to form nanoporous carbons with accessible N dopants to adsorb CO₂. The optimal materials were synthesized using N-heterocycle additives to control the amount of coordinated DMF in the base MOF structure, thereby increasing its thermal stability prior to pyrolysis.

Original language	English
Pages (from-to)	8015-8020
Number of pages	6
Journal	CrystEngComm
Volume	17
Issue number	42
DOIs	https://doi.org/10.1039/c5ce00828j
Publication status	Published - 2015

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Publisher Copyright:
© The Royal Society of Chemistry.

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10.1039/c5ce00828j

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abstract = "This paper describes the pyrolysis of pyridinedicarboxylate-containing Zn-based metal-organic frameworks (MOFs) to form nanoporous carbons with accessible N dopants to adsorb CO2. The optimal materials were synthesized using N-heterocycle additives to control the amount of coordinated DMF in the base MOF structure, thereby increasing its thermal stability prior to pyrolysis.",

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AU - Oliver, Allen G.

AU - Hicks, Jason C.

N1 - Publisher Copyright: © The Royal Society of Chemistry.

PY - 2015

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AB - This paper describes the pyrolysis of pyridinedicarboxylate-containing Zn-based metal-organic frameworks (MOFs) to form nanoporous carbons with accessible N dopants to adsorb CO2. The optimal materials were synthesized using N-heterocycle additives to control the amount of coordinated DMF in the base MOF structure, thereby increasing its thermal stability prior to pyrolysis.

UR - https://www.scopus.com/pages/publications/84945306381

U2 - 10.1039/c5ce00828j

DO - 10.1039/c5ce00828j

M3 - Article

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SN - 1466-8033

VL - 17

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JO - CrystEngComm

JF - CrystEngComm

IS - 42

ER -

Enhanced CO₂ capture capacities and efficiencies with N-doped nanoporous carbons synthesized from solvent-modulated, pyridinedicarboxylate-containing Zn-MOFs

Abstract

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