Pore-tuning to boost the electrocatalytic activity of polymeric micelle-templated mesoporous Pd nanoparticles

Cuiling Li; Muhammad Iqbal; Bo Jiang; Zhongli Wang; Jeonghun Kim; Ashok Kumar Nanjundan; Andrew E. Whitten; Kathleen Wood; Yusuke Yamauchi

doi:10.1039/C8SC03911A

Pore-tuning to boost the electrocatalytic activity of polymeric micelle-templated mesoporous Pd nanoparticles

Cuiling Li
, Muhammad Iqbal
, Bo Jiang
, Zhongli Wang
, Jeonghun Kim
, Ashok Kumar Nanjundan
, Andrew E. Whitten
, Kathleen Wood
, Yusuke Yamauchi

Research output: Contribution to journal › Article › peer-review

188 Citations (Scopus)

Abstract

Understanding how mesoporous noble metal architectures affect electrocatalytic performance is very important for the rational design and preparation of high-performance electrocatalysts. Herein, by using polymeric micelle-assembled structures as templates, mesoporous Pd nanoparticles with tunable porous constructions are synthesized by simply tuning the solvent compositions. The effect of porous Pd nanoparticles on the electrocatalytic performance is thoroughly studied. Their superior electrocatalytic activity can be attributed to the mass transport efficiency and open porous structures.

Original language	English
Pages (from-to)	4054-4061
Number of pages	8
Journal	Chemical Science
Volume	10
Issue number	14
DOIs	https://doi.org/10.1039/C8SC03911A
Publication status	Published - 14 Apr 2019

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© The Royal Society of Chemistry.

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abstract = "Understanding how mesoporous noble metal architectures affect electrocatalytic performance is very important for the rational design and preparation of high-performance electrocatalysts. Herein, by using polymeric micelle-assembled structures as templates, mesoporous Pd nanoparticles with tunable porous constructions are synthesized by simply tuning the solvent compositions. The effect of porous Pd nanoparticles on the electrocatalytic performance is thoroughly studied. Their superior electrocatalytic activity can be attributed to the mass transport efficiency and open porous structures.",

author = "Cuiling Li and Muhammad Iqbal and Bo Jiang and Zhongli Wang and Jeonghun Kim and Nanjundan, \{Ashok Kumar\} and Whitten, \{Andrew E.\} and Kathleen Wood and Yusuke Yamauchi",

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AU - Li, Cuiling

AU - Iqbal, Muhammad

AU - Jiang, Bo

AU - Wang, Zhongli

AU - Kim, Jeonghun

AU - Nanjundan, Ashok Kumar

AU - Whitten, Andrew E.

AU - Wood, Kathleen

AU - Yamauchi, Yusuke

PY - 2019/4/14

Y1 - 2019/4/14

N2 - Understanding how mesoporous noble metal architectures affect electrocatalytic performance is very important for the rational design and preparation of high-performance electrocatalysts. Herein, by using polymeric micelle-assembled structures as templates, mesoporous Pd nanoparticles with tunable porous constructions are synthesized by simply tuning the solvent compositions. The effect of porous Pd nanoparticles on the electrocatalytic performance is thoroughly studied. Their superior electrocatalytic activity can be attributed to the mass transport efficiency and open porous structures.

AB - Understanding how mesoporous noble metal architectures affect electrocatalytic performance is very important for the rational design and preparation of high-performance electrocatalysts. Herein, by using polymeric micelle-assembled structures as templates, mesoporous Pd nanoparticles with tunable porous constructions are synthesized by simply tuning the solvent compositions. The effect of porous Pd nanoparticles on the electrocatalytic performance is thoroughly studied. Their superior electrocatalytic activity can be attributed to the mass transport efficiency and open porous structures.

UR - https://www.scopus.com/pages/publications/85064035677

U2 - 10.1039/C8SC03911A

DO - 10.1039/C8SC03911A

M3 - Article

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JO - Chemical Science

JF - Chemical Science

IS - 14

ER -

Pore-tuning to boost the electrocatalytic activity of polymeric micelle-templated mesoporous Pd nanoparticles

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