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Solvent dependent photo-isomerization of 4-dimethylaminoazobenzene carboxylic acid

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Abstract

We have observed reversible trans-cis photo-isomerization behaviors of 4-dimethylaminoazobenzene carboxylic acid (4DAzC) in ethyl acetate by alternating irradiations at 370 and 430 nm. The photo-isomerization from trans- to cis-isomer was found to be strongly solvent dependent and not to occur efficiently in water and ethanol. Also photo-isomerization from cis- to trans-isomer was occurred upon 370 nm illumination or via thermal relaxation. The activation energy for the thermal isomerization from cis to trans-isomer was estimated to be 49.2 kJ/mol in ethyl acetate from the temperature-dependent kinetic absorption measurements.

Original languageEnglish
Pages (from-to)176-179
Number of pages4
JournalChemical Physics
Volume361
Issue number3
DOIs
Publication statusPublished - 15 Jul 2009

Keywords

  • Activation energy
  • Azobenzene
  • Cis-trans isomerization
  • Reversibility
  • Solvent effect
  • Temperature-dependent UV-Vis absorption spectroscopy

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